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Journal article

Tandem Ring-Closing Metathesis/Isomerization Reactions for the Total Synthesis of Violacein

By Petersen, Mette T.; Nielsen, Thomas E.

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Department of Chemistry

A series of 5-substituted 2-pyrrolidinones was synthesized through a one-pot ruthenium alkylidene-catalyzed tandem RCM/isomerization/nucleophilic addition sequence. The intermediates resulting from RCM/isomerization showed reactivity toward electrophiles in aldol condensation reactions which provided a new entry for the total synthesis of the antileukemic natural product violacein.

Language: English
Publisher: American Chemical Society
Year: 2013
Pages: 1986-1989
ISSN: 15237052 and 15237060
Types: Journal article
DOI: 10.1021/ol400654r

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