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Journal article

Tracking of Airborne Radionuclides from the Damaged Fukushima Dai-Ichi Nuclear Reactors by European Networks

From

Institut de radioprotection et de sûreté nucléaire1

Universitá degli Studi di Milano2

Icelandic Radiation Safety Authority3

Vienna University of Technology4

Health Protection Agency5

Radiological Protection Institute of Ireland6

Comenius University7

Radiological Monitoring and Data Acquisition Network8

Aristotle University of Thessaloniki9

Central Laboratory for Radiological Protection10

University of Belgrade11

Laruex12

Austrian Agency for Health and Food Safety GmbH13

Defence Forces Technical Research Centre14

Radiation and Nuclear Safety Authority15

National Institute of Public Health and the Environment16

Ministry of Health Luxembourg17

University College Dublin18

Norwegian Radiation Protection Authority19

Center for Physical Sciences and Technology20

National Radiation Protection Institute21

Radioecology and Tracer Studies, Radiation Research Division, Risø National Laboratory for Sustainable Energy, Technical University of Denmark22

Federal Office for Radiation Protection23

Radiation Research Division, Risø National Laboratory for Sustainable Energy, Technical University of Denmark24

Risø National Laboratory for Sustainable Energy, Technical University of Denmark25

Bulgarian Academy of Sciences26

International Atomic Energy Agency27

Republican Center of Radiation Control and Environment Monitoring28

The Danish Environmental Protection Agency29

Federal Agency for Nuclear Control30

Federal Office of Public Health31

University of Bologna32

Helmholtz Zentrum München - German Research Center for Environmental Health33

Polish Academy of Sciences34

Polytechnic University of Catalonia35

Physikalisch-Technische Bundesanstalt36

Italian Network for the Radioactivity Environmental Monitoring37

Instituto Tecnológico e Nuclear38

Babes-Bolyai University39

Deutscher Wetterdienst40

Swedish Defence Research Agency41

...and 31 more

Radioactive emissions into the atmosphere from the damaged reactors of the Fukushima Dai-ichi nuclear power plant (NPP) started on March 12th, 2011. Among the various radionuclides released, iodine-131 (131I) and cesium isotopes (137Cs and 134Cs) were transported across the Pacific toward the North American continent and reached Europe despite dispersion and washout along the route of the contaminated air masses.

In Europe, the first signs of the releases were detected 7 days later while the first peak of activity level was observed between March 28th and March 30th. Time variations over a 20-day period and spatial variations across more than 150 sampling locations in Europe made it possible to characterize the contaminated air masses.

After the Chernobyl accident, only a few measurements of the gaseous 131I fraction were conducted compared to the number of measurements for the particulate fraction. Several studies had already pointed out the importance of the gaseous 131I and the large underestimation of the total 131I airborne activity level, and subsequent calculations of inhalation dose, if neglected.

The measurements made across Europe following the releases from the Fukushima NPP reactors have provided a significant amount of new data on the ratio of the gaseous 131I fraction to total 131I, both on a spatial scale and its temporal variation. It can be pointed out that during the Fukushima event, the 134Cs to 137Cs ratio proved to be different from that observed after the Chernobyl accident.

The data set provided in this paper is the most comprehensive survey of the main relevant airborne radionuclides from the Fukushima reactors, measured across Europe. A rough estimate of the total 131I inventory that has passed over Europe during this period was

Language: English
Year: 2011
Pages: 7670-7677
ISSN: 15205851 and 0013936x
Types: Journal article
DOI: 10.1021/es2017158
ORCIDs: Nielsen, Sven Poul

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