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Journal article

Coherent Interaction of Three-Dimensionally Confined Electron-Hole Pairs with LO-Phonons

From

Department of Micro- and Nanotechnology, Technical University of Denmark1

The spectrally resolved FWM signal of CdSe quantum dots with sizes below the bulk excitonic Bohr radius has been studied as a function of temperature and excitation intensity and compared with bulk CdSe. A clear oscillation with a period of 163fs (approximate to 25 meV) is found in the transient FWM signal and attributed to a coherent coupling of confined electron-hole pairs with LO-phonons.

Two side bands are observed in the spectrum 25 meV below and above the excitonic resonance. The strong coupling to LO-phonons is observed even at excitation densities around 1 x 10(16) cm(-3) which is close to the bulk value of the Mott density.

Language: English
Publisher: WILEY-VCH Verlag
Year: 1997
Pages: 42-44
ISSN: 15213951 and 03701972
Types: Journal article
DOI: 10.1002/1521-3951(199711)204:1<42::AID-PSSB42>3.0.CO;2-P

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