Conference paper
Experiments and modeling of SNCR process in a cyclone reactor
CHEC Research Centre, Department of Chemical and Biochemical Engineering, Technical University of Denmark1
Department of Chemical and Biochemical Engineering, Technical University of Denmark2
The Hempel Foundation Coatings Science and Technology Centre (CoaST), Department of Chemical and Biochemical Engineering, Technical University of Denmark3
In this study, the SNCR process was investigated in a pilot scale cyclone reactor by experiments and modeling. Experiments were conducted under different conditions, with inlet gas temperatures of 850-1100 °C, inlet gas velocities of 12-15 m/s, NH3/NO feed molar ratios of 0-7, and with and without particle loading.
NOx reduction, ammonia slip, temperature, and concentration profiles inside the cyclone were measured. With a NO inlet concentration of 500 ppm, 90% NO reduction was achieved at inlet temperatures of 900-1000 °C and a NH3/NO ratio of approximately 3, but with ammonia slips of 150-300ppm. Measurements showed that the NO reduction took place mainly in the cyclone inlet, while ammonia converted further inside the cyclone, even in zones with temperatures significantly lower than the typicalSNCR window.
The system was modeled by reactor network models using detailed kinetics, and a modelthat could describe the internal concentration profiles was developed.
Language: | English |
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Year: | 2020 |
Proceedings: | Nordic Flame Days 2019 |
Types: | Conference paper |
ORCIDs: | Wu, Hao , Lin, Weigang and Dam-Johansen, Kim |