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Book chapter

Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond

In Structure and Bonding — 2012, pp. 185-211

By Møller, Klaus Braagaard1,2; Henriksen, Niels Engholm1,2

Edited by Mingos, David Michael P.; Dahl, Jens Peder; Day, Peter

From

Physical Chemistry, Department of Chemistry, Technical University of Denmark1

Department of Chemistry, Technical University of Denmark2

We review the basic theoretical formulation for pulsed X-ray scattering on nonstationary molecular states. Relevant time scales are discussed for coherent as well as incpherent X-ray pulses. The general formalism is applied to a nonstationary diatomic molecule in order to highlight the relation between the signal and the time-dependent quamtum distribution of internuclear positions.

Finally, a few experimental results are briefly discussed.

Language: English
Publisher: Springer
Year: 2012
Pages: 185-211
Series: Structure and Bonding
ISBN: 3642273696 , 364227370X , 364227370x , 9783642273698 and 9783642273704
ISSN: 16168550 and 00815993
Types: Book chapter
DOI: 10.1007/430_2011_58
ORCIDs: Møller, Klaus Braagaard and Henriksen, Niels Engholm
Keywords

Diatomic molecule Inversion Nonstationary states Pump probe X-ray scattering

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