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Journal article

A Polyphenylene Support for Pd Catalysts with Exceptional Catalytic Activity

By Wang, Feng1; Mielby, Jerrik Jørgen2,3; Richter, Felix Herrmann1; Wang, Guanghui1; Prieto, Gonzalo1; Kasama, Takeshi4; Weidenthaler, Claudia1; Bongard, Hans-Josef1; Kegnæs, Søren2,3; Fuerstner, Alois1; Schueth, Ferdi1 ...and 1 more

From

Max Planck Institute1

Department of Chemistry, Technical University of Denmark2

Centre for Catalysis and Sustainable Chemistry, Department of Chemistry, Technical University of Denmark3

Center for Electron Nanoscopy, Technical University of Denmark4

We describe a solid polyphenylene support that serves as an excellent platform for metal-catalyzed reactions that are normally carried out under homogeneous conditions. The catalyst is synthesized by palladium-catalyzed Suzuki coupling which directly results in formation of palladium nanoparticles confined to a porous polyphenylene network.

The composite solid is in turn highly active for further Suzuki coupling reactions, including non-activated substrates that are challenging even for molecular catalysts.

Language: English
Publisher: WILEY‐VCH Verlag
Year: 2014
Pages: 8645-8648
ISSN: 15213773 and 14337851
Types: Journal article
DOI: 10.1002/anie.201404912
ORCIDs: Mielby, Jerrik Jørgen , Kasama, Takeshi and Kegnæs, Søren
Keywords

cross-coupling cross‐coupling nanoparticles polymer supports polyphenylenes

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