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Journal article

Homogeneous and heterogeneously catalyzed oxidation of SO2

By Jørgensen, Tommy L.1; Livbjerg, Hans1; Glarborg, Peter2,3

From

Technical University of Denmark1

CHEC Research Centre, Department of Chemical and Biochemical Engineering, Technical University of Denmark2

Department of Chemical and Biochemical Engineering, Technical University of Denmark3

Oxidation of SO2-SO3 has been studied experimentally in laboratory flow reactors. The homogeneous oxidation by O2 was characterized in the temperature range 1023-1323K at semi-dry and moist conditions. The reaction was found to be very slow, in agreement with results from literature. The experimental data compared well with modeling predictions using a recently published reaction mechanism for gas-phase SO2 oxidation.

The ability of quartz, alumina and iron oxide to catalyze the SO2 oxidation was studied in the temperature range 873-1273K. Quartz was found to be inert to SO2 oxidation, while alumina promoted the oxidation. Iron oxide was found to be a strong oxidation catalyst, in agreement with results from literature.

Language: English
Year: 2007
Pages: 4496-4499
ISSN: 18734405 and 00092509
Types: Journal article
DOI: 10.1016/j.ces.2007.05.016
ORCIDs: Glarborg, Peter
Keywords

Catalysis Reaction mechanism SO2 SO3 Sulfuric acid

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