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Preprint article · Journal article

Dzyaloshinskii-Moriya interaction and the magnetic ground state in magnetoelectric LiCoPO4

From

Neutrons and X-rays for Materials Physics, Department of Physics, Technical University of Denmark1

Department of Physics, Technical University of Denmark2

Paul Scherrer Institute3

Imaging and Structural Analysis, Department of Energy Conversion and Storage, Technical University of Denmark4

Department of Energy Conversion and Storage, Technical University of Denmark5

Technical University of Denmark6

Iowa State University7

Magnetic structures are investigated by means of neutron diffraction to shine a light on the intricate details that are believed to be key to understanding the magnetoelectric effect in LiCoPO4. At zero field, a spontaneous spincanting of ϕ = 7(1)° is found. The spins tilt away from the easy b-axis toward c.

Symmetry considerations lead to the magnetic point group m'z, which is consistent with the previously observed magnetoelectric tensorform and weak ferromagnetic moment along b. For magnetic fields applied along a, the induced ferromagnetic moment couples via the Dzyaloshinskii-Moriya interaction to yield an additional field-induced spin canting.

An upper limitto the size of the interaction is estimated from the canting angle.

Language: English
Year: 2019
ISSN: 24699969 , 24699950 , 1550235x and 10980121
Types: Preprint article and Journal article
DOI: 10.1103/PhysRevB.99.104421
ORCIDs: 0000-0003-4118-5702 , Fogh, Ellen , Sørensen, Michael Korning , Christensen, Niels Bech and Toft-Petersen, Rasmus
Keywords

cond-mat.str-el

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