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Journal article

Multi-modal characterization of kesterite thin-film solar cells: experimental results and numerical interpretation

By Saadaldin, Abdellatif1; Slyamov, Azat M.2; Stuckelberger, Michael E.3; Jørgensen, Peter S.2,4; Rein, Christian2; Lucas, Mariana Mar2,5; Ramos, Tiago2; Rodriguez-Fernandez, Angel6; Bernard, Dominique1; Andreasen, Jens W.2,5

From

Université de Bordeaux1

Department of Energy Conversion and Storage, Technical University of Denmark2

German Electron Synchrotron3

Continuum Modelling and Testing, Department of Energy Conversion and Storage, Technical University of Denmark4

Imaging and Structural Analysis, Department of Energy Conversion and Storage, Technical University of Denmark5

Lund University6

We report a multi-modal study of the electrical, chemical and structural properties of a kesterite thin-film solar cell by combining the spatially-resolved X-ray beam induced current and fluorescence imaging techniques for the evaluation of a fully functional device on a cross-section. The data allowed the correlation of the chemical composition, defects at interfaces and inhomogeneous deposition of the layers with the local charge-collection efficiency of the device.

We support our observations with Monte Carlo simulations of high-energy X-ray interactions with the semiconductor device, and finite-volume modeling of the charge-collection efficiency.

Language: English
Publisher: The Royal Society of Chemistry
Year: 2022
Pages: 160-179
ISSN: 13645498 and 13596640
Types: Journal article
DOI: 10.1039/d2fd00044j
ORCIDs: Jørgensen, Peter S. , Rein, Christian , Andreasen, Jens W. , 0000-0002-8244-5235 and 0000-0001-6637-0731

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