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Journal article

Formation of acetic acid by aqueous-phase oxidation of ethanol with air in the presence of a heterogeneous gold catalyst

By Christensen, Claus H.1,2; Jørgensen, Betina3; Hansen, Jeppe Rass3; Egeblad, Kresten3; Madsen, Robert3; Kegnæs, Søren3,4; Hansen, Stine M.5; Hansen, Mike R.5; Andersen, Hans C.5

From

Administration, Department of Chemical and Biochemical Engineering, Technical University of Denmark1

Department of Chemical and Biochemical Engineering, Technical University of Denmark2

Department of Chemistry, Technical University of Denmark3

Sustainable and Green Chemistry, Department of Chemistry, Technical University of Denmark4

Technical University of Denmark5

Wine into vinegar: It is possible to selectively oxidize ethanol into acetic acid in aqueous solution with air as the oxidant and a heterogeneous gold catalyst (see TEM image of supported gold particles) at temperatures of about 423 K and O2 pressures of 0.6 MPa. This reaction proceeds readily in aqueous acidic media with yields of up to 90 % and CO2 as the only major by-product.

Language: English
Publisher: WILEY-VCH Verlag
Year: 2006
Pages: 4648-4651
ISSN: 05700833 , 15213773 and 14337851
Types: Journal article
DOI: 10.1002/anie.200601180
ORCIDs: Madsen, Robert and Kegnæs, Søren
Keywords

acetic acid bioethanol gold heterogeneous catalysis oxidation

Other keywords

Acetic Acid Air Catalysis Ethanol Gold Oxidation-Reduction

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