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Preprint article · Journal article

Dimensional evolution of spin correlations in the magnetic pyrochlore Yb2Ti2O7

From

McMaster University1

University of Waterloo2

Nano-Microstructures in Materials, Materials Research Division, Risø National Laboratory for Sustainable Energy, Technical University of Denmark3

Materials Research Division, Risø National Laboratory for Sustainable Energy, Technical University of Denmark4

Risø National Laboratory for Sustainable Energy, Technical University of Denmark5

Indiana University-Purdue University Indianapolis6

University of Maryland, College Park7

Los Alamos National Laboratory8

The pyrochlore material Yb2Ti2O7 displays unexpected quasi-two-dimensional (2D) magnetic correlations within a cubic lattice environment at low temperatures, before entering an exotic disordered ground state below T=265 mK. We report neutron scattering measurements of the thermal evolution of the 2D spin correlations in space and time.

Short-range three-dimensional (3D) spin correlations develop below 400 mK, accompanied by a suppression in the quasielastic (QE) scattering below ∼0.2 meV. These show a slowly fluctuating ground state with spins correlated over short distances within a kagome-triangular-kagome (KTK) stack along [111], which evolves to isolated kagome spin stars at higher temperatures.

Furthermore, low-temperature specific heat results indicate a sample dependence to the putative transition temperature that is bounded by 265 mK, which we discuss in the context of recent mean field theoretical analysis. ©2011 American Physical Society

Language: English
Year: 2011
Pages: 5
ISSN: 1550235x , 10980121 , 24699950 and 01631829
Types: Preprint article and Journal article
DOI: 10.1103/PhysRevB.84.174442
Keywords

cond-mat.str-el

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