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Journal article · Preprint article

Electron and phonon drag in thermoelectric transport through coherent molecular conductors

From

Huazhong University of Science and Technology1

National University of Singapore2

University of Copenhagen3

Center for Nanostructured Graphene, Centers, Technical University of Denmark4

Department of Micro- and Nanotechnology, Technical University of Denmark5

Theoretical Nanoelectronics, Department of Micro- and Nanotechnology, Technical University of Denmark6

We study thermoelectric transport through a coherent molecular conductor connected to two electron and two phonon baths using the nonequilibrium Green's function method. We focus on the mutual drag between electron and phonon transport as a result of ‘momentum’ transfer, which happens only when there are at least two phonon degrees of freedom.

After deriving expressions for the linear drag coefficients, obeying the Onsager relation, we further investigate their effect on nonequilibrium transport. We show that the drag effect is closely related to two other phenomena: (1) adiabatic charge pumping through a coherent conductor; (2) the current-induced nonconservative and effective magnetic forces on phonons.

Language: English
Year: 2016
ISSN: 24699969 , 24699950 , 1550235x and 10980121
Types: Journal article and Preprint article
DOI: 10.1103/PhysRevB.93.205404
ORCIDs: Brandbyge, Mads and 0000-0002-6328-7462

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