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Journal article

Selective production of hydrogen peroxide and oxidation of hydrogen sulfide in an unbiased solar photoelectrochemical cell

By Zong, Xu1; Chen, Hongjun1; Seger, Brian2,3; Pedersen, Thomas4,5; Dargusch, Matthew S.1; McFarland, Eric W.; Li, Can6; Wang, Lianzhou1

From

University of Queensland1

Department of Physics, Technical University of Denmark2

Surface Physics and Catalysis, Department of Physics, Technical University of Denmark3

Department of Micro- and Nanotechnology, Technical University of Denmark4

Silicon Microtechnology, Department of Micro- and Nanotechnology, Technical University of Denmark5

Chinese Academy of Sciences6

A solar-to-chemical conversion process is demonstrated using a photoelectrochemical cell without external bias for selective oxidation of hydrogen sulfide (H2S) to produce hydrogen peroxide (H2O2) and sulfur (S). The process integrates two redox couples anthraquinone/anthrahydroquinone and I−/I3−, and conceptually illustrates the remediation of a waste product for producing valuable chemicals.

Language: English
Publisher: The Royal Society of Chemistry
Year: 2014
Pages: 3347-3351
ISSN: 17545706 and 17545692
Types: Journal article
DOI: 10.1039/C4EE01503G
ORCIDs: Seger, Brian and Pedersen, Thomas

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